Absolutely! You can cancel your plan at any time. You'll be entitled to your services until your next billing date, when your services will stop.
The lowdown:
Log in to the app and go to the Your Profile section (top right icon)
Go to the Cancel your plan section and follow the instructions.
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Alternatively you can cancel your plan by logging in to your account at https://simpmobile.com/login
π Keep in mind that whilst cancelling is completely free, you will lose all your coins and unredeemed rewards.